In January 2011, Ilonzeh was announced as one of the "Angels" on the reboot of the 1970s television series Charlie's Angels. The series, which premiered in September 2011, received mostly negative reviews, and was cancelled the day after the fourth episode. In March 2012, it was announced that Ilonzeh would be recurring on The CW series Arrow. Later that year, she began appearing in a recurring role in the ABC Family drama series Switched at Birth. In 2013, she played a leading role in the Lifetime television film Killer Reality. Ilonzeh also guest starred in the second season of CW's Beauty & the Beast, and had a recurring role on Lifetime comedy-drama Drop Dead Diva in 2013. Later, she had a recurring roles on Person of Interest and Empire.